CSAR Seminar

SPEAKER: Alexander Telengator, University of California at San Diego

TITLE: Several Models in Combustion of Porous Energetic Materials

DATE: Friday, August 25, 2006
TIME: 10:00 A.M.
PLACE: 2240 DCL
1304 W. Springfield Ave., Urbana, IL

ABSTRACT

Combustion processes in energetic materials are of interest in the fields of pyrotechnics, gas generation and most importantly, propulsion. There are a number of various types of propellants based on their composition. In the problems presented here, we address such energetic materials as nitramines, where both the fuel and oxidizer are contained in the same molecule.

Pristine energetic materials degrade over time, resulting in a porous-propellant scenario. Safety and burning characteristics of such a degraded propellant will be considerably affected not only by porosity itself but by two-phase flow effects. A relative motion between the gas and condensed phases in both the solid-gas preheat region, bubbling melt layer as well as the exothermic reaction region is a fundamental aspect of multiphase deflagration in porous energetic materials. Our models of multiphase burning processes in porous solid propellants belong to a more general field of heterogeneous combustion.

Various intermediate phases exist in the context of solid-propellant burning, such as, for example, bubbling melt layers and a dispersed phase. There are models that assume a scenario where a gaseous flame is preceded simply by sublimation and/or pyrolysis reactions. In the context of 'unconfined' quasi-steady deflagrations, the approximation of small Mach number may imply that the gas pressure is independent of the spatial coordinate. However, under certain conditions, a confinement in the system may arise, thus causing a significant difference between the upstream and downstream values of the gas pressure, or overpressure. Consequently, growing overpressure leads to a rapid increase in the burning rate; i.e., a transition from conductive to convective burning.

In the problems described here, we addressed several models in combustion of porous solid propellants under confinement. The global combustion mechanism is adopted as a condensed-phase reaction (bubbling melt layer, sublimation and/or partial pyrolysis) followed by a gaseous flame to form the final gas-phase products.